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Sten Yngve Dennis Lagergren (6 May 1876 – 4 April 1922) was a Swedish physical chemist known for his fundamental findings in
adsorption Adsorption is the adhesion of atoms, ions or molecules from a gas, liquid or dissolved solid to a surface. This process creates a film of the ''adsorbate'' on the surface of the ''adsorbent''. This process differs from absorption, in which ...
kinetics Kinetics ( grc, κίνησις, , kinesis, ''movement'' or ''to move'') may refer to: Science and medicine * Kinetics (physics), the study of motion and its causes ** Rigid body kinetics, the study of the motion of rigid bodies * Chemical k ...
. Lagergrens's 1898 article "Zur Theorie der Sogenannten Adsorption Gelöster Stoffe" (To the theory of the so-called adsorption of dissolved materials) brought him a lasting fame. In 2018, 120 years after its publication, the paper was cited more than 800 times according to Clarivate Analytics' Web of Science, making its total number of citation above 6000. In addition, his name became an
eponym An eponym is a person, a place, or a thing after whom or which someone or something is, or is believed to be, named. The adjectives which are derived from the word eponym include ''eponymous'' and ''eponymic''. Usage of the word The term ''epon ...
in the form of ''Lagergren equation'' or ''Lagergren kinetics'' occurring several thousand times in the literature.


Biography


Early life

Sten Lagergren was born in Ramnäs, Sweden on 6 May 1876. His father, Per Henrik Lagergren, was a commercial agent, his mother was Hilda Amalia Vistrand.


Education and professional career

Lagergren attended to the university college Stockholms Högskola (Stockholm Highschool; the predecessor of the present
Stockholm University Stockholm University ( sv, Stockholms universitet) is a public research university in Stockholm, Sweden, founded as a college in 1878, with university status since 1960. With over 33,000 students at four different faculties: law, humanities, s ...
), and studied there between 1894 and 1899. He wrote the paper that made him famous as a university student. Apparently, it made him a "one hit wonder", since no other notable scientific paper have been written by him anymore. He became a secondary school teacher, and was the rector of the Sofi Almquists samskola from 1902 and of the Beskowska skolan between 1905 and 1913. He was the author of several secondary school textbooks in geometry.


Marriage and children

Lagergren married Alfhild Lindström (born in 1877) in 1906. They had one daughter.


Death

Sten Lagergren died on 4 April 1922 in
Lidingö Lidingö, also known in its definite form ''Lidingön'' and as ''Lidingölandet'', is an island in the inner Stockholm archipelago, northeast of Stockholm, Sweden. In 2010, the population of the Lidingö urban area on the island was 31,561. It ...
, Sweden.


His classic work and its aftermath

In his perennial 1898 paper, Lagergren formulated a so-called pseudo-first-order model for adsorption kinetics based on an extensive body of experimental measurements. Both the empirical data and the model were highly acclaimed by the contemporaries. In 1900,
Wilhelm Ostwald Friedrich Wilhelm Ostwald (; 4 April 1932) was a Baltic German chemist and philosopher. Ostwald is credited with being one of the founders of the field of physical chemistry, with Jacobus Henricus van 't Hoff, Walther Nernst, and Svante Arrh ...
(Nobel Prize winner in Chemistry in 1909) wrote an unusually extensive review of the paper in his Zeitschrift für physikalische Chemie. Beyond words of recognition, Ostwald also drafted some ideas to further develop the model. Actually, having abandoned research, Lagergren could not give thought to these advises. The path was followed, instead, by
Herbert Freundlich Herbert Max Finlay Freundlich (28 January 1880 in Charlottenburg – 30 March 1941 in Minneapolis) was a German chemist. His father was of German Jewish descent, and his mother ( Finlay) was from Scotland. His younger brother was Erw ...
. His paper based on his habilitation lecture heavily relies upon Lagergren's results. They were also included in his classic book, in its later editions, and since then, in all standard treatises of surface chemistry and related areas. The first occurrence of the eponymic use of Lagergren's name can be traced back to an article of Dietl ("Lagergren'sche Formel" on p. 800). The use of Lagergren's model gained a new impetus in the beginning of the 21st century largely with the advent of sorption-based technologies of water desalination. A citation review of Lagergren's equation counted about 170 papers citing Lagergren's original paper until 2004. Within 10 years, this number exhibited a twentyfold increase.


Notes and references

{{DEFAULTSORT:Lagergren, Sten 20th-century chemists Swedish physical chemists 1876 births 1922 deaths 19th-century Swedish scientists 20th-century Swedish scientists 19th-century Swedish chemists Stockholm University alumni People from Surahammar Municipality