Frequency-resolved Optical Gating
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Frequency-resolved Optical Gating
Frequency-resolved optical gating (FROG) is a general method for measuring the spectral phase of ultrashort laser pulses, which range from sub femtosecond to about a nanosecond in length. Invented in 1991 by Rick Trebino and Daniel J. Kane, FROG was the first technique to solve this problem, which is difficult because, ordinarily, to measure an event in time, a shorter event is required with which to measure it. For example, to measure a soap bubble popping requires a strobe light with a shorter duration to freeze the action. Because ultrashort laser pulses are the shortest events ever created, before FROG, it was thought by many that their complete measurement in time was not possible. FROG, however, solved the problem by measuring an "auto-spectrogram" of the pulse, in which the pulse gates itself in a nonlinear-optical medium and the resulting gated piece of the pulse is then spectrally resolved as a function of the delay between the two pulses. Retrieval of the pulse from its ...
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Ultrashort Pulse
In optics, an ultrashort pulse, also known as an ultrafast event, is an electromagnetic pulse whose time duration is of the order of a picosecond (10−12 second) or less. Such pulses have a broadband optical spectrum, and can be created by mode-locked oscillators. Amplification of ultrashort pulses almost always requires the technique of chirped pulse amplification, in order to avoid damage to the gain medium of the amplifier. They are characterized by a high peak intensity (or more correctly, irradiance) that usually leads to nonlinear interactions in various materials, including air. These processes are studied in the field of nonlinear optics. In the specialized literature, "ultrashort" refers to the femtosecond (fs) and picosecond (ps) range, although such pulses no longer hold the record for the shortest pulses artificially generated. Indeed, x-ray pulses with durations on the attosecond time scale have been reported. The 1999 Nobel Prize in Chemistry was awarded ...
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Second-harmonic Generation
Second-harmonic generation (SHG, also called frequency doubling) is a nonlinear optical process in which two photons with the same frequency interact with a nonlinear material, are "combined", and generate a new photon with twice the energy of the initial photons (equivalently, twice the frequency and half the wavelength), that conserves the coherence of the excitation. It is a special case of sum-frequency generation (2 photons), and more generally of harmonic generation. The second-order nonlinear susceptibility of a medium characterizes its tendency to cause SHG. Second-harmonic generation, like other even-order nonlinear optical phenomena, is not allowed in media with inversion symmetry (in the leading electric dipole contribution). However, effects such as the Bloch–Siegert shift (oscillation), found when two-level systems are driven at Rabi frequencies comparable to their transition frequencies, will give rise to second harmonic generation in centro-symmetric systems. ...
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Nonlinear Optics
Nonlinear optics (NLO) is the branch of optics that describes the behaviour of light in ''nonlinear media'', that is, media in which the polarization density P responds non-linearly to the electric field E of the light. The non-linearity is typically observed only at very high light intensities (when the electric field of the light is >108 V/m and thus comparable to the atomic electric field of ~1011 V/m) such as those provided by lasers. Above the Schwinger limit, the vacuum itself is expected to become nonlinear. In nonlinear optics, the superposition principle no longer holds. History The first nonlinear optical effect to be predicted was two-photon absorption, by Maria Goeppert Mayer for her PhD in 1931, but it remained an unexplored theoretical curiosity until 1961 and the almost simultaneous observation of two-photon absorption at Bell Labs and the discovery of second-harmonic generation by Peter Franken ''et al.'' at University of Michigan, both shortly after the constru ...
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Review Of Scientific Instruments
''Review of Scientific Instruments'' is a monthly peer-reviewed scientific journal published by the American Institute of Physics. Its area of interest is scientific instruments, apparatus, and techniques. According to the ''Journal Citation Reports'', the journal has a 2018 impact factor The impact factor (IF) or journal impact factor (JIF) of an academic journal is a scientometric index calculated by Clarivate that reflects the yearly mean number of citations of articles published in the last two years in a given journal, as i ... of 1.587. References External links * Chemistry journals Physics journals Research methods journals American Institute of Physics academic journals Monthly journals English-language journals {{physics-journal-stub ...
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Multiphoton Intrapulse Interference Phase Scan
Multiphoton intrapulse interference phase scan (MIIPS) is a method used in ultrashort laser technology that simultaneously measures (phase characterization), and compensates (phase correction) femtosecond laser pulses using an adaptive pulse shaper. When an ultrashort laser pulse reaches a duration of less than a few hundred femtosecond, it becomes critical to characterize its duration, its temporal intensity curve, or its electric field as a function of time. Classical photodetectors measuring the intensity of light are still too slow to allow for a direct measurement, even with the fastest photodiodes or streak cameras. Other means have been developed based on quasi instantaneous non linear optical effects such as autocorrelation, FROG, SPIDER, etc. However, these can only measure the pulse characteristics but not correct for defects in order to make the pulse as short as possible. For instance, the pulse could be linearly chirped or present higher order group delay dispersion (G ...
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Spectral Phase Interferometry For Direct Electric-field Reconstruction
In ultrafast optics, spectral phase interferometry for direct electric-field reconstruction (SPIDER) is an ultrashort pulse measurement technique originally developed by Chris Iaconis and Ian Walmsley. The basics SPIDER is an interferometric ultrashort pulse measurement technique in the frequency domain based on spectral shearing interferometry. Spectral shearing interferometry is similar in concept to lateral shearing interferometry, except the shearing is performed in the frequency domain. The spectral shear is typically generated by sum-frequency mixing the test pulse with two different quasi-monochromatic frequencies (usually derived by chirping a copy of the pulse itself), although it can also be achieved by spectral filtering or even with linear electro-optic modulators for picosecond pulses. The interference between the two upconverted pulses allows the spectral phase at one frequency to be referenced to the spectral phase at a different frequency, separated by the spectral ...
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Double-Blind FROG
Double-blind frequency-resolved optical gating (double-blind FROG) is a method for simultaneously measuring two unknown ultrashort laser pulses. Well established ultrafast measurement techniques such as frequency-resolved optical gating and its simplified version GRENOUILLE can only measure one unknown ultrashort laser pulse at a time. Another version of FROG, called cross-correlation FROG (XFROG), also measures only one pulse, but it involves two pulses: a known reference pulse and the unknown pulse to be measured. In modern optics experiments, ultrashort laser pulses have been used in a great variety of engineering application and scientific research, for example, biomedical engineering, material science, nonlinear spectroscopy, ultrafast chemistry, etc. Often, these experiments involve using two potentially different input laser pulses, for example, Raman spectroscopy, two-color pump-probe experiments, and non-degenerate four-wave mixing. In many situations, an output pulse is ...
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Grating-eliminated No-nonsense Observation Of Ultrafast Incident Laser Light E-fields
Grating-eliminated no-nonsense observation of ultrafast incident laser light e-fields (GRENOUILLE) is an ultrashort pulse measurement technique based on frequency-resolved optical gating (FROG). The acronym was chosen because of the technique's relationship to FROG; ''grenouille'' is French for ''frog''. Theory Because most FROG techniques have an autocorrelator, they also have the sensitive alignment issues that come with it. In addition, most FROGs use a thin second-harmonic generation (SHG) crystal and a spectrometer, adding signal strength requirements as well as additional alignment issues. GRENOUILLE is a simple device based on the SHG FROG, replacing the beam splitter, delay line and beam recombination components of the autocorrelator with a prism, and replacing the spectrometer and thin SHG crystal combination with a thick SHG crystal. The effect of these replacements is to eliminate all sensitive alignment parameters while increasing the signal strength. These changes als ...
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Overdetermined System
In mathematics, a system of equations is considered overdetermined if there are more equations than unknowns. An overdetermined system is almost always inconsistent (it has no solution) when constructed with random coefficients. However, an overdetermined system will have solutions in some cases, for example if some equation occurs several times in the system, or if some equations are linear combinations of the others. The terminology can be described in terms of the concept of constraint counting. Each unknown can be seen as an available degree of freedom. Each equation introduced into the system can be viewed as a constraint that restricts one degree of freedom. Therefore, the critical case occurs when the number of equations and the number of free variables are equal. For every variable giving a degree of freedom, there exists a corresponding constraint. The ''overdetermined'' case occurs when the system has been overconstrained — that is, when the equations outnumb ...
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Diffraction Grating
In optics, a diffraction grating is an optical component with a periodic structure that diffracts light into several beams travelling in different directions (i.e., different diffraction angles). The emerging coloration is a form of structural coloration. The directions or diffraction angles of these beams depend on the wave (light) incident angle to the diffraction grating, the spacing or distance between adjacent diffracting elements (e.g., parallel slits for a transmission grating) on the grating, and the wavelength of the incident light. The grating acts as a dispersive element. Because of this, diffraction gratings are commonly used in monochromators and spectrometers, but other applications are also possible such as optical encoders for high precision motion control and wavefront measurement. For typical applications, a reflective grating has ridges or ''rulings'' on its surface while a transmissive grating has transmissive or hollow slits on its surface. Such a grating ...
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Femtosecond
A femtosecond is a unit of time in the International System of Units (SI) equal to 10 or of a second; that is, one quadrillionth, or one millionth of one billionth, of a second. For context, a femtosecond is to a second as a second is to about 31.71 million years; a ray of light travels approximately 0.3  μm (micrometers) in 1 femtosecond, a distance comparable to the diameter of a virus.Compared with overview in: Page 3 The word ''femtosecond'' is formed by the SI prefix ''femto'' and the SI unit ''second''. Its symbol is fs. A femtosecond is equal to 1000 attoseconds, or 1/1000 picosecond. Because the next higher SI unit is 1000 times larger, times of 10−14 and 10−13 seconds are typically expressed as tens or hundreds of femtoseconds. * Typical time steps for molecular dynamics simulations are on the order of 1 fs. * The periods of the waves of visible light have a duration of about 2 femtoseconds. = = 2.0 \times 10^~ The precise duration depends on the ener ...
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