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Spallation is a process in which fragments of material (
spall Spall are fragments of a material that are broken off a larger solid body. It can be produced by a variety of mechanisms, including as a result of projectile impact, corrosion, weathering, cavitation, or excessive rolling pressure (as in a ball ...
) are ejected from a body due to impact or stress. In the context of impact mechanics it describes ejection of material from a target during impact by a
projectile A projectile is an object that is propelled by the application of an external force and then moves freely under the influence of gravity and air resistance. Although any objects in motion through space are projectiles, they are commonly found i ...
. In planetary physics, spallation describes
meteor A meteoroid () is a small rocky or metallic body in outer space. Meteoroids are defined as objects significantly smaller than asteroids, ranging in size from grains to objects up to a meter wide. Objects smaller than this are classified as mi ...
itic impacts on a planetary surface and the effects of
stellar wind A stellar wind is a flow of gas ejected from the upper atmosphere of a star. It is distinguished from the bipolar outflows characteristic of young stars by being less collimated, although stellar winds are not generally spherically symmetric. ...
s and
cosmic rays Cosmic rays are high-energy particles or clusters of particles (primarily represented by protons or atomic nuclei) that move through space at nearly the speed of light. They originate from the Sun, from outside of the Solar System in our ...
on planetary atmospheres and surfaces. In the context of
mining Mining is the extraction of valuable minerals or other geological materials from the Earth, usually from an ore body, lode, vein, seam, reef, or placer deposit. The exploitation of these deposits for raw material is based on the econom ...
or
geology Geology () is a branch of natural science concerned with Earth and other Astronomical object, astronomical objects, the features or rock (geology), rocks of which it is composed, and the processes by which they change over time. Modern geology ...
, spallation can refer to pieces of rock breaking off a rock face due to the internal stresses in the rock; it commonly occurs on
mine shaft Shaft mining or shaft sinking is the action of excavating a mine shaft from the top down, where there is initially no access to the bottom. Shallow shafts, typically sunk for civil engineering projects, differ greatly in execution method from ...
walls. In the context of
anthropology Anthropology is the scientific study of humanity, concerned with human behavior, human biology, cultures, societies, and linguistics, in both the present and past, including past human species. Social anthropology studies patterns of be ...
, spallation is a process used to make stone tools such as arrowheads by knapping. In
nuclear physics Nuclear physics is the field of physics that studies atomic nuclei and their constituents and interactions, in addition to the study of other forms of nuclear matter. Nuclear physics should not be confused with atomic physics, which studies t ...
, spallation is the process in which a heavy nucleus emits numerous nucleons as a result of being hit by a high-energy
particle In the physical sciences, a particle (or corpuscule in older texts) is a small localized object which can be described by several physical or chemical properties, such as volume, density, or mass. They vary greatly in size or quantity, from ...
, thus greatly reducing its atomic weight. In industrial processes and bioprocessing the loss of tubing material due to the repeated flexing of the tubing within a peristaltic pump is termed spallation.


In solid mechanics

Spallation can occur when a tensile stress wave propagates through a material and can be observed in flat plate impact tests. It is caused by an internal cavitation due to stresses, which are generated by the interaction of stress waves, exceeding the local
tensile strength Ultimate tensile strength (UTS), often shortened to tensile strength (TS), ultimate strength, or F_\text within equations, is the maximum stress that a material can withstand while being stretched or pulled before breaking. In brittle materials ...
of materials. A fragment or multiple fragments will be created on the free end of the plate. This fragment known as "
spall Spall are fragments of a material that are broken off a larger solid body. It can be produced by a variety of mechanisms, including as a result of projectile impact, corrosion, weathering, cavitation, or excessive rolling pressure (as in a ball ...
" acts as a secondary projectile with velocities that can be as high as one third of the stress wave speed on the material. This type of failure is typically an effect of high explosive squash head ( HESH) charges.


Laser spallation

Laser induced spallation is a recent experimental technique developed to understand the
adhesion Adhesion is the tendency of dissimilar particles or surfaces to cling to one another ( cohesion refers to the tendency of similar or identical particles/surfaces to cling to one another). The forces that cause adhesion and cohesion can ...
of thin films with substrates. A high energy pulsed
laser A laser is a device that emits light through a process of optical amplification based on the stimulated emission of electromagnetic radiation. The word "laser" is an acronym for "light amplification by stimulated emission of radiation". The ...
(typically Nd:YAG) is used to create a compressive stress pulse in the substrate wherein it propagates and reflects as a tensile wave at the free boundary. This tensile pulse spalls/peels the thin film while propagating towards the substrate. Using theory of
wave propagation Wave propagation is any of the ways in which waves travel. Single wave propagation can be calculated by 2nd order wave equation ( standing wavefield) or 1st order one-way wave equation. With respect to the direction of the oscillation relative ...
in solids it is possible to extract the interface strength. The stress pulse created in this example is usually around 3-8 nanoseconds in duration while its magnitude varies as a function of
laser A laser is a device that emits light through a process of optical amplification based on the stimulated emission of electromagnetic radiation. The word "laser" is an acronym for "light amplification by stimulated emission of radiation". The ...
fluence. Due to the non-contact application of load, this technique is very well suited to spall ultra- thin films (1 micrometre in thickness or less). It is also possible to mode convert a longitudinal stress wave into a
shear stress Shear stress, often denoted by ( Greek: tau), is the component of stress coplanar with a material cross section. It arises from the shear force, the component of force vector parallel to the material cross section. '' Normal stress'', on ...
using a pulse shaping prism and achieve shear spallation.


Nuclear spallation

Nuclear spallation occurs naturally in
Earth's atmosphere The atmosphere of Earth is the layer of gases, known collectively as air, retained by Earth's gravity that surrounds the planet and forms its planetary atmosphere. The atmosphere of Earth protects life on Earth by creating pressure allowing fo ...
owing to the impacts of
cosmic ray Cosmic rays are high-energy particles or clusters of particles (primarily represented by protons or atomic nuclei) that move through space at nearly the speed of light. They originate from the Sun, from outside of the Solar System in our own ...
s, and also on the surfaces of bodies in space such as
meteorite A meteorite is a solid piece of debris from an object, such as a comet, asteroid, or meteoroid, that originates in outer space and survives its passage through the atmosphere to reach the surface of a planet or moon. When the original object ...
s and the
Moon The Moon is Earth's only natural satellite. It is the fifth largest satellite in the Solar System and the largest and most massive relative to its parent planet, with a diameter about one-quarter that of Earth (comparable to the width of ...
. Evidence of cosmic ray spallation (also known as "spoliation") is seen on outer surfaces of bodies, and gives a means of measuring the length of time of exposure. The composition of the cosmic rays themselves also indicates that they have suffered spallation before reaching Earth, because the proportion of light elements such as lithium, boron, and beryllium in them exceeds average cosmic abundances; these elements in the cosmic rays were evidently formed from spallation of oxygen, nitrogen, carbon and perhaps silicon in the cosmic ray sources or during their lengthy travel here. ''Cosmogenic''
isotopes Isotopes are two or more types of atoms that have the same atomic number (number of protons in their nuclei) and position in the periodic table (and hence belong to the same chemical element), and that differ in nucleon numbers ( mass numbers ...
of
aluminium Aluminium (aluminum in American and Canadian English) is a chemical element with the symbol Al and atomic number 13. Aluminium has a density lower than those of other common metals, at approximately one third that of steel. It ha ...
,
beryllium Beryllium is a chemical element with the symbol Be and atomic number 4. It is a steel-gray, strong, lightweight and brittle alkaline earth metal. It is a divalent element that occurs naturally only in combination with other elements to for ...
,
chlorine Chlorine is a chemical element with the symbol Cl and atomic number 17. The second-lightest of the halogens, it appears between fluorine and bromine in the periodic table and its properties are mostly intermediate between them. Chlorine i ...
,
iodine Iodine is a chemical element with the Symbol (chemistry), symbol I and atomic number 53. The heaviest of the stable halogens, it exists as a semi-lustrous, non-metallic solid at standard conditions that melts to form a deep violet liquid at , ...
and neon, formed by spallation of terrestrial elements under cosmic ray bombardment, have been detected on Earth. Nuclear spallation is one of the processes by which a particle accelerator may be used to produce a beam of
neutron The neutron is a subatomic particle, symbol or , which has a neutral (not positive or negative) charge, and a mass slightly greater than that of a proton. Protons and neutrons constitute the atomic nucleus, nuclei of atoms. Since protons and ...
s. A particle beam consisting of protons at around 1 GeV are shot into a target consisting of mercury,
tantalum Tantalum is a chemical element with the symbol Ta and atomic number 73. Previously known as ''tantalium'', it is named after Tantalus, a villain in Greek mythology. Tantalum is a very hard, ductile, lustrous, blue-gray transition metal that ...
,
lead Lead is a chemical element with the symbol Pb (from the Latin ) and atomic number 82. It is a heavy metal that is denser than most common materials. Lead is soft and malleable, and also has a relatively low melting point. When freshly cut, ...
or another heavy metal. The target nuclei are excited and upon deexcitation, 20 to 30 neutrons are expelled per nucleus. Although this is a far more expensive way of producing neutron beams than by a chain reaction of
nuclear fission Nuclear fission is a reaction in which the nucleus of an atom splits into two or more smaller nuclei. The fission process often produces gamma photons, and releases a very large amount of energy even by the energetic standards of radio ...
in a
nuclear reactor A nuclear reactor is a device used to initiate and control a fission nuclear chain reaction or nuclear fusion reactions. Nuclear reactors are used at nuclear power plants for electricity generation and in nuclear marine propulsion. Heat fr ...
, it has the advantage that the beam can be pulsed with relative ease. Furthermore, the energetic cost of one spallation neutron is six times lower than that of a neutron gained via nuclear fission. In contrast to nuclear fission, the spallation neutrons cannot trigger further spallation or fission processes to produce further neutrons. Therefore, there is no chain reaction, which makes the process non-critical. Observations of cosmic ray spallation had already been made in the 1930s, but the first observations from a particle accelerator occurred in 1947, and the term "spallation" was coined by Nobelist Glenn T. Seaborg that same year. Spallation is a proposed neutron source in subcritical nuclear reactors like the upcoming research reactor MYRRHA, which is planned to investigate the feasibility of
nuclear transmutation Nuclear transmutation is the conversion of one chemical element or an isotope into another chemical element. Nuclear transmutation occurs in any process where the number of protons or neutrons in the nucleus of an atom is changed. A transmutatio ...
of high level waste into less harmful substances. Besides having a neutron multiplication factor ''just below'' criticality, subcritical reactors can also produce net usable energy as the average energy expenditure per neutron produced ranges around 30 MeV (1GeV beam producing a bit over 30 neutrons in the most productive targets) while fission produces on the order of 200 MeV per actinide atom that is split. Even at relatively low energy efficiency of the processes involved, net usable energy could be generated while being able to use actinides unsuitable for use in conventional reactors as "fuel".


Production of neutrons at a spallation neutron source

Generally the production of neutrons at a spallation source begins with a high-powered proton accelerator. The accelerator may consist of a linac only (as in the
European Spallation Source The European Spallation Source ERIC (ESS) is a multi-disciplinary research facility based on the world's most powerful pulsed neutron source. It is currently under construction in Lund, Sweden. The ESS Data Management and Software Centre (DMS ...
) or a combination of linac and synchrotron (e.g. ISIS neutron source) or a cyclotron (e.g. SINQ (PSI)) . As an example, the ISIS neutron source is based on some components of the former Nimrod synchrotron. Nimrod was uncompetitive for
particle physics Particle physics or high energy physics is the study of fundamental particles and forces that constitute matter and radiation. The fundamental particles in the universe are classified in the Standard Model as fermions (matter particles) an ...
so it was replaced with a new synchrotron, initially using the original
injector An injector is a system of ducting and nozzles used to direct the flow of a high-pressure fluid in such a way that a lower pressure fluid is entrained in the jet and carried through a duct to a region of higher pressure. It is a fluid-dynamic ...
s, but which produces a highly intense pulsed beam of protons. Whereas Nimrod would produce around 2 µA at 7 GeV, ISIS produces 200 µA at 0.8 GeV. This is pulsed at the rate of 50 Hz, and this intense beam of protons is focused onto a target. Experiments have been done with
depleted uranium Depleted uranium (DU; also referred to in the past as Q-metal, depletalloy or D-38) is uranium with a lower content of the fissile isotope than natural uranium.: "Depleted uranium possesses only 60% of the radioactivity of natural uranium, hav ...
targets but although these produce the most intense neutron beams, they also have the shortest lives. Generally, therefore,
tantalum Tantalum is a chemical element with the symbol Ta and atomic number 73. Previously known as ''tantalium'', it is named after Tantalus, a villain in Greek mythology. Tantalum is a very hard, ductile, lustrous, blue-gray transition metal that ...
or
tungsten Tungsten, or wolfram, is a chemical element with the symbol W and atomic number 74. Tungsten is a rare metal found naturally on Earth almost exclusively as compounds with other elements. It was identified as a new element in 1781 and first isol ...
targets have been used. Spallation processes in the target produce the neutrons, initially at very high energies—a good fraction of the proton energy. These neutrons are then slowed in moderators filled with
liquid hydrogen Liquid hydrogen (LH2 or LH2) is the liquid state of the element hydrogen. Hydrogen is found naturally in the molecular H2 form. To exist as a liquid, H2 must be cooled below its critical point of 33  K. However, for it to be in a fully l ...
or liquid
methane Methane ( , ) is a chemical compound with the chemical formula (one carbon atom bonded to four hydrogen atoms). It is a group-14 hydride, the simplest alkane, and the main constituent of natural gas. The relative abundance of methane ...
to the energies that are needed for the scattering instruments. Whilst protons can be focused since they have charge, chargeless neutrons cannot be, so in this arrangement the instruments are arranged around the moderators. Inertial confinement fusion has the potential to produce orders of magnitude more neutrons than spallation. This could be useful for neutron radiography, which can be used to locate hydrogen atoms in structures, resolve atomic thermal motion, and study collective excitations of photons more effectively than
X-rays An X-ray, or, much less commonly, X-radiation, is a penetrating form of high-energy electromagnetic radiation. Most X-rays have a wavelength ranging from 10 picometers to 10 nanometers, corresponding to frequencies in the range 30&nbs ...
.


See also

*
Energy amplifier In nuclear physics, an energy amplifier is a novel type of nuclear power reactor, a subcritical reactor, in which an energetic particle beam is used to stimulate a reaction, which in turn releases enough energy to power the particle accelerator and ...
* Subcritical reactor (accelerator-driven system)


Spallation facilities

*
European Spallation Source The European Spallation Source ERIC (ESS) is a multi-disciplinary research facility based on the world's most powerful pulsed neutron source. It is currently under construction in Lund, Sweden. The ESS Data Management and Software Centre (DMS ...
, under construction, Sweden * ISIS neutron source, Harwell, UK * J-PARC * LANSCE Los Alamos * PSI Spallation Neutron Source (SINQ), Switzerland *
Spallation Neutron Source The Spallation Neutron Source (SNS) is an accelerator-based neutron source facility in the U.S. that provides the most intense pulsed neutron beams in the world for scientific research and industrial development.In 2007, SNS was entered into th ...
Oak Ridge, USA * China Spallation Neutron Source


References

{{Reflist


External links


IAEA database of spallation neutron sources
in th
Accelerator Knowledge Portal
technical background.

at the ISIS neutron and muon source Nuclear technology Neutron sources